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The outcomes reveal that straight graphene sheets and you will nanocrystalline diamonds alternatively come, in which straight graphene sheets develop to the a lot of time ribbons and you will graphite needles, and in the end change to the diamonds. A changeover techniques away from graphite (200) in order to diamond (110) verifies the newest sales, and you can Ta atoms from gorgeous filaments can be found in order to atomically move in the video clips. First concept calculations make sure Ta-added H- otherwise O-terminated bilayer graphene in an instant turns to the diamond. Which implies that on the H, O, and Ta cutting-edge environment of the CVD ecosystem, diamond is formed by the phase conversion away from graphite. So it subverts all round degree one to graphite are etched by the hydrogen and you will sp3 carbon dioxide species accumulate in order to create diamond and you can provides a means to get ready large-area expensive diamonds considering higher-sized graphite under typical pressure.
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In these development process, the fresh hydrogen resource is switched off, and the carbon dioxide origin try restored to one hundred sccm. Then, the growth power diminished in order to zero at a rate of 1 V/s to your closed carbon resource. HRTEM photos out of examples increasing (A)–(A-2) 0 s, (B)–(B-2) 29 s, (C)–(C-2) sixty s, (D)–(D-2) 90 s, (E)–(E-2) 120 s, (F)–(F-2) 150 s, (G)–(G-2) 180 s, and (H)–(H-2) 210 s within the 2nd development processes from the step 1,800 W. All of the white-dotted-line boxes are the section corresponding to the fresh inset FFT pictures.
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